It would depend on what you already have.
If you don't have a strong Blissey, then I think that would top the list for me. She can be a good defender and a good attacker.
If that is your only Tyranitar then that would be next on the list.
...and can I assume the other is a Lapras?
I am sure you already know it is capable of destrying a couple of DNites as it is, so this would be less of a priority.
So in this order...
Blissey
T-Rex
Lapras
...unless you already have a stable full of any one of them.
EDIT I did not see the pic before I posted...as you have a good Blissey, I would be tempted to work the T-Rex first.